N‐Acyliminium Ion Chemistry: Highly Efficient and Versatile Carbon–Carbon Bond Formation by Nucleophilic Substitution of Hydroxy Groups Catalyzed by Sn(NTf2)4
Identifieur interne : 000995 ( Main/Exploration ); précédent : 000994; suivant : 000996N‐Acyliminium Ion Chemistry: Highly Efficient and Versatile Carbon–Carbon Bond Formation by Nucleophilic Substitution of Hydroxy Groups Catalyzed by Sn(NTf2)4
Auteurs : Raja Ben Thman [Tunisie] ; Radouane Affani ; Marie-José Tranchant ; Sylvain Antoniotti ; Vincent Dalla [France] ; Elisabet Du Ach [France]Source :
- Angewandte Chemie [ 0044-8249 ] ; 2010-01-18.
English descriptors
- KwdEn :
Abstract
Atomökonomisch: Nichtmodifizierte N,O‐Halbacetale wurden in einer katalytischen, hocheffizienten α‐Amidoalkylierung kohlenstoffzentrierter Nucleophile eingesetzt, darunter Siliciumverbindungen, aktive Methylenderivate, elektronenreiche Arene und selbst einfache Ketone (siehe Schema). In der Regel genügt 1 Mol‐% des supersauren Lewis‐Reagens Sn(NTf2)4 als Katalysator.
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DOI: 10.1002/ange.200906036
Affiliations:
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<front><div type="abstract">Atomökonomisch: Nichtmodifizierte N,O‐Halbacetale wurden in einer katalytischen, hocheffizienten α‐Amidoalkylierung kohlenstoffzentrierter Nucleophile eingesetzt, darunter Siliciumverbindungen, aktive Methylenderivate, elektronenreiche Arene und selbst einfache Ketone (siehe Schema). In der Regel genügt 1 Mol‐% des supersauren Lewis‐Reagens Sn(NTf2)4 als Katalysator.</div>
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